TY - JOUR
T1 - Universality of the Nonphononic Vibrational Spectrum across Different Classes of Computer Glasses
AU - Richard, David
AU - Gonzalez-Lopez, Karina
AU - Kapteijns, Geert
AU - Pater, Robert
AU - Vaknin, Talya
AU - Bouchbinder, Eran
AU - Lerner, Edan
N1 - We wish to acknowledge inspiring discussions with Itamar Procaccia, Corrado Rainone, and Yuri Lubomirsky. D. R. acknowledges support of the Simons Foundation for the “Cracking the Glass Problem Collaboration” Grant No. 348126. K. G.-L. acknowledges the computer resources provided by the Laboratorio Nacional del Sureste de México, CONACYT member of the national laboratories network. E. L. acknowledges support from the NWO (Vidi Grant No. 680-47-554/3259). E. B. acknowledges support from the Minerva Foundation with funding from the Federal German Ministry for Education and Research, the Ben May Center for Chemical Theory and Computation, and the Harold Perlman Family.
PY - 2020/8/21
Y1 - 2020/8/21
N2 - It has been recently established that the low-frequency spectrum of simple computer glass models is populated by soft, quasilocalized nonphononic vibrational modes whose frequencies ω follow a gapless, universal distribution D(ω)∼ω4. While this universal nonphononic spectrum has been shown to be robust to varying the glass history and spatial dimension, it has so far only been observed in simple computer glasses featuring radially symmetric, pairwise interaction potentials. Consequently, the relevance of the universality of nonphononic spectra seen in simple computer glasses to realistic laboratory glasses remains unclear. Here, we demonstrate the emergence of the universal ω4 nonphononic spectrum in a broad variety of realistic computer glass models, ranging from tetrahedral network glasses with three-body interactions, through molecular glasses and glassy polymers, to bulk metallic glasses. Taken together with previous observations, our results indicate that the low-frequency nonphononic vibrational spectrum of any glassy solid quenched from a melt features the universal ω4 law, independently of the nature of its microscopic interactions.
AB - It has been recently established that the low-frequency spectrum of simple computer glass models is populated by soft, quasilocalized nonphononic vibrational modes whose frequencies ω follow a gapless, universal distribution D(ω)∼ω4. While this universal nonphononic spectrum has been shown to be robust to varying the glass history and spatial dimension, it has so far only been observed in simple computer glasses featuring radially symmetric, pairwise interaction potentials. Consequently, the relevance of the universality of nonphononic spectra seen in simple computer glasses to realistic laboratory glasses remains unclear. Here, we demonstrate the emergence of the universal ω4 nonphononic spectrum in a broad variety of realistic computer glass models, ranging from tetrahedral network glasses with three-body interactions, through molecular glasses and glassy polymers, to bulk metallic glasses. Taken together with previous observations, our results indicate that the low-frequency nonphononic vibrational spectrum of any glassy solid quenched from a melt features the universal ω4 law, independently of the nature of its microscopic interactions.
UR - http://www.scopus.com/inward/record.url?scp=85090820319&partnerID=8YFLogxK
U2 - 10.1103/PhysRevLett.125.085502
DO - 10.1103/PhysRevLett.125.085502
M3 - مقالة
SN - 0031-9007
VL - 125
JO - Physical review letters
JF - Physical review letters
IS - 8
M1 - 085502
ER -