TY - JOUR
T1 - Universal Nonphononic Density of States in 2D, 3D, and 4D Glasses
AU - Kapteijns, Geert
AU - Bouchbinder, Eran
AU - Lerner, Edan
N1 - E. L. acknowledges support from the Netherlands Organisation for Scientific Research (NWO) (Vidi Grant No. 680-47-554/3259). E. B. acknowledges support from the Minerva Foundation with funding from the Federal German Ministry for Education and Research, the William Z. and Eda Bess Novick Young Scientist Fund, and the Harold Perlman Family.
PY - 2018/8/3
Y1 - 2018/8/3
N2 - It is now well established that structural glasses possess disorder- and frustration-induced soft quasilocalized excitations, which play key roles in various glassy phenomena. Recent work has established that in model glass formers in three dimensions, these nonphononic soft excitations may assume the form of quasilocalized, harmonic vibrational modes whose frequency follows a universal density of states D(ω)∼ω4, independently of microscopic details, and for a broad range of glass preparation protocols. Here, we further establish the universality of the nonphononic density of vibrational modes by direct measurements in model structural glasses in two dimensions and four dimensions. We also investigate their degree of localization, which is generally weaker in lower spatial dimensions, giving rise to a pronounced system-size dependence of the nonphononic density of states in two dimensions, but not in higher dimensions. Finally, we identify a fundamental glassy frequency scale ωc above which the universal ω4 law breaks down.
AB - It is now well established that structural glasses possess disorder- and frustration-induced soft quasilocalized excitations, which play key roles in various glassy phenomena. Recent work has established that in model glass formers in three dimensions, these nonphononic soft excitations may assume the form of quasilocalized, harmonic vibrational modes whose frequency follows a universal density of states D(ω)∼ω4, independently of microscopic details, and for a broad range of glass preparation protocols. Here, we further establish the universality of the nonphononic density of vibrational modes by direct measurements in model structural glasses in two dimensions and four dimensions. We also investigate their degree of localization, which is generally weaker in lower spatial dimensions, giving rise to a pronounced system-size dependence of the nonphononic density of states in two dimensions, but not in higher dimensions. Finally, we identify a fundamental glassy frequency scale ωc above which the universal ω4 law breaks down.
U2 - https://doi.org/10.1103/PhysRevLett.121.055501
DO - https://doi.org/10.1103/PhysRevLett.121.055501
M3 - مقالة
C2 - 30118293
SN - 0031-9007
VL - 121
JO - Physical review letters
JF - Physical review letters
IS - 5
M1 - 055501
ER -