Ultrafast Transverse Modulation of Free Electrons by Interaction with Shaped Optical Fields

Ivan Madan; Veronica Leccese; Adam Mazur; Francesco Barantani; Thomas Lagrange; Alexey Sapozhnik; Phoebe M. Tengdin; Simone Gargiulo; Enzo Rotunno; Jean Christophe Olaya; Ido Kaminer; Vincenzo Grillo; F. Javier García De Abajo; Fabrizio Carbone; Giovanni Maria Vanacore

doi:10.1021/acsphotonics.2c00850

Ultrafast Transverse Modulation of Free Electrons by Interaction with Shaped Optical Fields

Ivan Madan, Veronica Leccese, Adam Mazur, Francesco Barantani, Thomas Lagrange, Alexey Sapozhnik, Phoebe M. Tengdin, Simone Gargiulo, Enzo Rotunno, Jean Christophe Olaya, Ido Kaminer, Vincenzo Grillo, F. Javier García De Abajo, Fabrizio Carbone, Giovanni Maria Vanacore

Technion - Israel Institute of Technology

Research output: Contribution to journal › Article › peer-review

Abstract

Spatiotemporal electron-beam shaping is a bold frontier of electron microscopy. Over the past decade, shaping methods evolved from static phase plates to low-speed electrostatic and magnetostatic displays. Recently, a swift change of paradigm utilizing light to control free electrons has emerged. Here, we experimentally demonstrate arbitrary transverse modulation of electron beams without complicated electron-optics elements or material nanostructures, but rather using shaped light beams. On-demand spatial modulation of electron wavepackets is obtained via inelastic interaction with transversely shaped ultrafast light fields controlled by an external spatial light modulator. We illustrate this method for the cases of Hermite-Gaussian and Laguerre-Gaussian modulation and discuss their use in enhancing microscope sensitivity. Our approach dramatically widens the range of patterns that can be imprinted on the electron profile and greatly facilitates tailored electron-beam shaping.

Original language	English
Pages (from-to)	3215-3224
Number of pages	10
Journal	ACS Photonics
Volume	9
Issue number	10
DOIs	https://doi.org/10.1021/acsphotonics.2c00850
State	Published - 19 Oct 2022

Keywords

PINEM
electron-beam shaping
electron-photon interaction
spatial light modulator
ultrafast transmission electron microscopy

All Science Journal Classification (ASJC) codes

Electronic, Optical and Magnetic Materials
Biotechnology
Atomic and Molecular Physics, and Optics
Electrical and Electronic Engineering

Access to Document

10.1021/acsphotonics.2c00850

Cite this

Madan, I., Leccese, V., Mazur, A., Barantani, F., Lagrange, T., Sapozhnik, A., Tengdin, P. M., Gargiulo, S., Rotunno, E., Olaya, J. C., Kaminer, I., Grillo, V., De Abajo, F. J. G., Carbone, F., & Vanacore, G. M. (2022). Ultrafast Transverse Modulation of Free Electrons by Interaction with Shaped Optical Fields. ACS Photonics, 9(10), 3215-3224. https://doi.org/10.1021/acsphotonics.2c00850

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title = "Ultrafast Transverse Modulation of Free Electrons by Interaction with Shaped Optical Fields",

abstract = "Spatiotemporal electron-beam shaping is a bold frontier of electron microscopy. Over the past decade, shaping methods evolved from static phase plates to low-speed electrostatic and magnetostatic displays. Recently, a swift change of paradigm utilizing light to control free electrons has emerged. Here, we experimentally demonstrate arbitrary transverse modulation of electron beams without complicated electron-optics elements or material nanostructures, but rather using shaped light beams. On-demand spatial modulation of electron wavepackets is obtained via inelastic interaction with transversely shaped ultrafast light fields controlled by an external spatial light modulator. We illustrate this method for the cases of Hermite-Gaussian and Laguerre-Gaussian modulation and discuss their use in enhancing microscope sensitivity. Our approach dramatically widens the range of patterns that can be imprinted on the electron profile and greatly facilitates tailored electron-beam shaping.",

keywords = "PINEM, electron-beam shaping, electron-photon interaction, spatial light modulator, ultrafast transmission electron microscopy",

author = "Ivan Madan and Veronica Leccese and Adam Mazur and Francesco Barantani and Thomas Lagrange and Alexey Sapozhnik and Tengdin, \{Phoebe M.\} and Simone Gargiulo and Enzo Rotunno and Olaya, \{Jean Christophe\} and Ido Kaminer and Vincenzo Grillo and \{De Abajo\}, \{F. Javier Garc{\'i}a\} and Fabrizio Carbone and Vanacore, \{Giovanni Maria\}",

year = "2022",

month = oct,

day = "19",

doi = "10.1021/acsphotonics.2c00850",

language = "الإنجليزيّة",

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journal = "ACS Photonics",

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publisher = "American Chemical Society",

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Madan, I, Leccese, V, Mazur, A, Barantani, F, Lagrange, T, Sapozhnik, A, Tengdin, PM, Gargiulo, S, Rotunno, E, Olaya, JC, Kaminer, I, Grillo, V, De Abajo, FJG, Carbone, F & Vanacore, GM 2022, 'Ultrafast Transverse Modulation of Free Electrons by Interaction with Shaped Optical Fields', ACS Photonics, vol. 9, no. 10, pp. 3215-3224. https://doi.org/10.1021/acsphotonics.2c00850

TY - JOUR

T1 - Ultrafast Transverse Modulation of Free Electrons by Interaction with Shaped Optical Fields

AU - Madan, Ivan

AU - Leccese, Veronica

AU - Mazur, Adam

AU - Barantani, Francesco

AU - Lagrange, Thomas

AU - Sapozhnik, Alexey

AU - Tengdin, Phoebe M.

AU - Gargiulo, Simone

AU - Rotunno, Enzo

AU - Olaya, Jean Christophe

AU - Kaminer, Ido

AU - Grillo, Vincenzo

AU - De Abajo, F. Javier García

AU - Carbone, Fabrizio

AU - Vanacore, Giovanni Maria

PY - 2022/10/19

Y1 - 2022/10/19

N2 - Spatiotemporal electron-beam shaping is a bold frontier of electron microscopy. Over the past decade, shaping methods evolved from static phase plates to low-speed electrostatic and magnetostatic displays. Recently, a swift change of paradigm utilizing light to control free electrons has emerged. Here, we experimentally demonstrate arbitrary transverse modulation of electron beams without complicated electron-optics elements or material nanostructures, but rather using shaped light beams. On-demand spatial modulation of electron wavepackets is obtained via inelastic interaction with transversely shaped ultrafast light fields controlled by an external spatial light modulator. We illustrate this method for the cases of Hermite-Gaussian and Laguerre-Gaussian modulation and discuss their use in enhancing microscope sensitivity. Our approach dramatically widens the range of patterns that can be imprinted on the electron profile and greatly facilitates tailored electron-beam shaping.

AB - Spatiotemporal electron-beam shaping is a bold frontier of electron microscopy. Over the past decade, shaping methods evolved from static phase plates to low-speed electrostatic and magnetostatic displays. Recently, a swift change of paradigm utilizing light to control free electrons has emerged. Here, we experimentally demonstrate arbitrary transverse modulation of electron beams without complicated electron-optics elements or material nanostructures, but rather using shaped light beams. On-demand spatial modulation of electron wavepackets is obtained via inelastic interaction with transversely shaped ultrafast light fields controlled by an external spatial light modulator. We illustrate this method for the cases of Hermite-Gaussian and Laguerre-Gaussian modulation and discuss their use in enhancing microscope sensitivity. Our approach dramatically widens the range of patterns that can be imprinted on the electron profile and greatly facilitates tailored electron-beam shaping.

KW - PINEM

KW - electron-beam shaping

KW - electron-photon interaction

KW - spatial light modulator

KW - ultrafast transmission electron microscopy

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DO - 10.1021/acsphotonics.2c00850

M3 - مقالة

SN - 2330-4022

VL - 9

SP - 3215

EP - 3224

JO - ACS Photonics

JF - ACS Photonics

IS - 10

ER -

Ultrafast Transverse Modulation of Free Electrons by Interaction with Shaped Optical Fields

Abstract

Keywords

All Science Journal Classification (ASJC) codes

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