Ultrafast Terahertz Gating of the Polarization and Giant Nonlinear Optical Response in BiFeO3 Thin Films

Frank Chen; John Goodfellow; Shi Liu; Ilya Grinberg; Matthias C. Hoffmann; Anoop R. Damodaran; Yi Zhu; Peter Zalden; Xiaohang Zhang; Ichiro Takeuchi; Andrew M. Rappe; Lane W. Martin; Haidan Wen; Aaron M. Lindenberg

doi:https://doi.org/10.1002/adma.201502975

Ultrafast Terahertz Gating of the Polarization and Giant Nonlinear Optical Response in BiFeO₃ Thin Films

Frank Chen, John Goodfellow, Shi Liu, Ilya Grinberg, Matthias C. Hoffmann, Anoop R. Damodaran, Yi Zhu, Peter Zalden, Xiaohang Zhang, Ichiro Takeuchi, Andrew M. Rappe, Lane W. Martin, Haidan Wen, Aaron M. Lindenberg

Research output: Contribution to journal › Article › peer-review

Abstract

Terahertz pulses are applied as an all-optical bias to ferroelectric thin-film BiFeO₃ while monitoring the time-dependent ferroelectric polarization through its nonlinear optical response. Modulations in the intensity of the second harmonic light generated by the film correspond to on-off ratios of 220× gateable on femtosecond timescales. Polarization modulations comparable to the built-in static polarization are observed.

Original language	English
Pages (from-to)	6371-6375
Number of pages	5
Journal	Advanced Materials
Volume	27
Issue number	41
DOIs	https://doi.org/10.1002/adma.201502975
State	Published - 4 Nov 2015
Externally published	Yes

Keywords

ferroelectrics
nonlinear optical properties
terahertz modulators
ultra-fast

All Science Journal Classification (ASJC) codes

Mechanics of Materials
Mechanical Engineering
General Materials Science

Access to Document

https://doi.org/10.1002/adma.201502975

Cite this

Chen, F., Goodfellow, J., Liu, S., Grinberg, I., Hoffmann, M. C., Damodaran, A. R., Zhu, Y., Zalden, P., Zhang, X., Takeuchi, I., Rappe, A. M., Martin, L. W., Wen, H., & Lindenberg, A. M. (2015). Ultrafast Terahertz Gating of the Polarization and Giant Nonlinear Optical Response in BiFeO₃ Thin Films. Advanced Materials, 27(41), 6371-6375. https://doi.org/10.1002/adma.201502975

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abstract = "Terahertz pulses are applied as an all-optical bias to ferroelectric thin-film BiFeO3 while monitoring the time-dependent ferroelectric polarization through its nonlinear optical response. Modulations in the intensity of the second harmonic light generated by the film correspond to on-off ratios of 220× gateable on femtosecond timescales. Polarization modulations comparable to the built-in static polarization are observed.",

keywords = "ferroelectrics, nonlinear optical properties, terahertz modulators, ultra-fast",

author = "Frank Chen and John Goodfellow and Shi Liu and Ilya Grinberg and Hoffmann, {Matthias C.} and Damodaran, {Anoop R.} and Yi Zhu and Peter Zalden and Xiaohang Zhang and Ichiro Takeuchi and Rappe, {Andrew M.} and Martin, {Lane W.} and Haidan Wen and Lindenberg, {Aaron M.}",

note = "Publisher Copyright: {\textcopyright} 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.",

year = "2015",

month = nov,

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doi = "https://doi.org/10.1002/adma.201502975",

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T1 - Ultrafast Terahertz Gating of the Polarization and Giant Nonlinear Optical Response in BiFeO3 Thin Films

AU - Chen, Frank

AU - Goodfellow, John

AU - Liu, Shi

AU - Grinberg, Ilya

AU - Hoffmann, Matthias C.

AU - Damodaran, Anoop R.

AU - Zhu, Yi

AU - Zalden, Peter

AU - Zhang, Xiaohang

AU - Takeuchi, Ichiro

AU - Rappe, Andrew M.

AU - Martin, Lane W.

AU - Wen, Haidan

AU - Lindenberg, Aaron M.

PY - 2015/11/4

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AB - Terahertz pulses are applied as an all-optical bias to ferroelectric thin-film BiFeO3 while monitoring the time-dependent ferroelectric polarization through its nonlinear optical response. Modulations in the intensity of the second harmonic light generated by the film correspond to on-off ratios of 220× gateable on femtosecond timescales. Polarization modulations comparable to the built-in static polarization are observed.

KW - ferroelectrics

KW - nonlinear optical properties

KW - terahertz modulators

KW - ultra-fast

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