Abstract
The microscopic modeling of spin-orbit entangled j=1/2 Mott insulators such as the layered hexagonal iridates Na2IrO3 and Li2IrO3 has spurred an interest in the physics of Heisenberg-Kitaev models. Here we explore the effect of lattice distortions on the formation of the collective spin-orbital states that include not only conventionally ordered phases but also gapped and gapless spin-orbital liquids. In particular, we demonstrate that in the presence of distortions, i.e., spatial anisotropies of the exchange couplings, conventionally ordered states are formed through an order-by-disorder selection, which is not only sensitive to the type of exchange anisotropy but also to the relative strength of the Heisenberg and Kitaev couplings. The spin-orbital liquid phases of the Kitaev limit - a gapless phase in the vicinity of spatially isotropic couplings and a gapped Z2 phase for a dominant spatial anisotropy of the exchange couplings - show vastly different sensitivities to the inclusion of a Heisenberg exchange. While the gapless phase is remarkably stable, the gapped Z2 phase quickly breaks down in what might be a rather unconventional phase transition driven by the simultaneous condensation of its elementary excitations.
| Original language | English |
|---|---|
| Article number | 035113 |
| Journal | Physical Review B - Condensed Matter and Materials Physics |
| Volume | 90 |
| Issue number | 3 |
| DOIs | |
| State | Published - 14 Jul 2014 |
All Science Journal Classification (ASJC) codes
- Electronic, Optical and Magnetic Materials
- Condensed Matter Physics