Abstract
Nonequilibrium thermodynamics of the driven resonant-level model is studied using numerical simulations based on the driven Liouville von-Neumann formalism. The approach is first validated against recently obtained analytical results for quasistatic level shifts and the corresponding first-order corrections. The numerical approach is then used to study far-from-equilibrium thermodynamic properties of the system under finite level shift rates. The proposed methodology allows the study of unexplored nonequilibrium thermodynamic regimes in open quantum systems.
Original language | English |
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Pages (from-to) | 1232-1248 |
Number of pages | 17 |
Journal | Journal of Chemical Theory and Computation |
Volume | 16 |
Issue number | 2 |
DOIs | |
State | Published - 11 Feb 2020 |
All Science Journal Classification (ASJC) codes
- Computer Science Applications
- Physical and Theoretical Chemistry