Abstract
We theoretically explore a scheme for generation of bright circularly and elliptically polarized high-order harmonics by bursts of linearly polarized pulses with a rotating polarization axis. Circularly polarized harmonics are formed if the bursts are comprised of N pulses that uphold an N-fold rotational symmetry, for N > 2. Rotating the polarization axes of the comprising pulses can generate elliptical harmonics with a collectively tunable ellipticity, from circular through elliptic to linear. The method preserves the single-cycle, single-atom and macroscopic physics of 'standard' linearly polarized high harmonic generation, with a high yield and cutoff energy. We investigate the method from a time-domain perspective, as well as a photonic perspective, and formulate the energy and spin-angular momentum conservation laws for this scheme. We find that the case of N = 4 is optimal for this method, resulting with the highest conversion efficiency of elliptical photons. The new features of this source offer new applications to helical ultrafast spectroscopy and ellipsometry.
| Original language | English |
|---|---|
| Article number | 31 |
| Journal | Photonics |
| Volume | 4 |
| Issue number | 2 |
| DOIs | |
| State | Published - 1 Jun 2017 |
Keywords
- Dynamical symmetry
- High harmonic generation
- UV optics
- Ultrafast spectroscopy
All Science Journal Classification (ASJC) codes
- Atomic and Molecular Physics, and Optics
- Instrumentation
- Radiology Nuclear Medicine and imaging
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