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An exchange-based diagnostic for static correlation

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

Abstract

We propose here a DFT-based diagnostic for static correlation %TAEX [TPSS@HF - HF] which effectively measures how different the DFT and HF exchange energies for a given HF density are. This and %TAEcorr[TPSS] are two cost-effective a priori estimates for the adequacy of the importance of static correlation. %TAEX[TPSS@HF - HF] contains nearly the same information as the earlier A diagnostic, but may be more intuitive to understand. Principal component and variable clustering analyses of a large number of static correlation diagnostics reveal that much of the variation is explained by just two components, and almost all of it by four; these are blocked by four variable clusters (single excitations; correlation entropy; double excitations; pragmatic energetics).
Original languageEnglish GB
Title of host publicationInternational Conference of Computational Methods in Sciences and Engineering, ICCMSE 2021
EditorsTheodore Simos, Charalambos Tsitouras, Zacharoula Kalogiratou, Theodore Monovasilis
PublisherAmerican Institute of Physics
ISBN (Electronic)9780735442474
DOIs
StatePublished - 23 Nov 2022
EventInternational Conference of Computational Methods in Sciences and Engineering 2021, ICCMSE 2021 - Heraklion, Greece
Duration: 4 Sep 20217 Sep 2021

Publication series

NameAIP Conference Proceedings
Volume2611
ISSN (Print)0094-243X

Conference

ConferenceInternational Conference of Computational Methods in Sciences and Engineering 2021, ICCMSE 2021
Country/TerritoryGreece
CityHeraklion
Period4/09/217/09/21

ASJC Scopus subject areas

  • General Physics and Astronomy

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